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Water Chemistry of the Unconsolidated Deposits of the Metro East, Illinois area

                                                                                                                                     

HERBICIDES, THEIR TRANSFORMATION PRODUCTS, AND ANTIBIOTICS:

           GROUND-WATER QUALITY DATA FOR THE METRO EAST, ILLINOIS AREA

 

During August-October 2005, the U.S. Geological Survey (USGS) conducted a synoptic study of agricultural

chemicals in ground water in the St. Louis metropolitan area counties of Madison and St. Clair, Illinois

(often referred to as the Metro East area). Samples from 6 monitoring wells and 2 public-supply wells were

analyzed for 6 acetamide herbicides (acetochlor, alachlor, dimethenamid, flufenacet, metolachlor, and

propachlor) and 26 of their transformation products (often referred to as degradates or metabolites).

Additionally, a sample from one monitoring well in the area was analyzed for antibiotic compounds.

 

The wells were selected to provide increased understanding of the extent of these compounds in the source

waters used for public supply in the region.  Past analyses for acetamide transformation products in the area

 is limited to a single set of samples from three additional public-supply wells (Mills and McMillan, 2004).

Review of available data indicates no previous antibiotic analyses. All wells were open to unconsolidated

deposits that range in composition from clay and silt to sand and gravel. Well depths ranged from about 17

to 112 feet; depth to ground water ranged from about 3.5 to 33.2 feet.  The public-supply wells and two

of the monitoring wells were open to the alluvial aquifer underlying the part of the Metro East area

referred to as the American Bottoms. All the wells sampled for herbicides were located within 0.25 mile of

land in current or past row-crop production. The well sampled for antibiotics was open to generally fine-

grained deposits that compose the uplands west of the American Bottoms; the well is located within 100 yards

of a sanitary sewer main, a commercial development, a residential street and subdivision, and a state highway.

 

 

Details regarding sampling methodology are given in Kolpin and Burkart (1991) and Mills and McMillan (2002). 

Water samples were collected using field-parameter stabilization and volumetric purge criteria to ensure

samples were representative of the aquifer water quality. Samples from water-supply wells were collected

before water treatment (chlorination, for example). All samples were filtered through a 0.7 micron baked

glass-fiber filter, chilled immediately to 4 degrees Centigrade, and shipped to the laboratory within 2 days of

collection.

 

Analyses were made at the USGS Organic Geochemistry Research Laboratory in Lawrence, Kans. Acetamide

compounds were analyzed by liquid chromatography/mass spectrometry (LC/MS) (Zimmerman and others, 2000;

Lee and others,  2001; and Lee and Strahan, 2003), as were antibiotic compounds (Lindsey and others, 2001).

 

 

The acetamide-herbicide and antibiotic analytical results from this study are given below. Additionally, related

herbicide results from these and other monitoring wells (William S. Morrow, U.S. Geological Survey, written

commun., 2006) and public-supply wells in the area (Mills and McMillan, 2004) are given.

              

 


References:

 

 

              

Kolpin, D.W., and Burkhart, M.R., 1991, Workplan for regional reconnaissance for selected

               herbicides and nitrate in ground water of the mid-continent United States, 1991:

               U.S. Geological Survey Open-File Report 91-59, 18 p.

 

Lee, E.A., Kish, J.L., Zimmerman, L.R., and Thurman, E.M., 2001, Method of analysis by the

               U.S. Geological Survey Organic Geochemistry Research Group - update and additions

        to the determination of chloroacetanilide herbicide degradation compounds in water

        using high-performance liquid chromatography/mass spectrometry: U.S. Geological

        Survey Open-File Report 01-10, 17 p.

        

Lee, E.A. and Strahan, A.P., 2003, Methods of analysis by the U.S. Geological Survey Organic

               Geochemistry Research Group - determination of acetamide herbicides and their

               degradation products in water using online solid-phase extraction and high-performance

               liquid chromatography/mass spectrometry: U.S. Geological Survey Open-File Report

               03-173, 17 p.

       

Lindsey, M.E., Meyer, M.T., and Thurman, E.M., 2001, Analysis of trace levels of sulfonamide

               and tetracycline antimicrobials in groundwater and surface water using solid-phase

               extraction and Liquid Chromatography/Mass Spectrometry, Analytical Chemistry, v. 74,

               p. 4640-4646.

              

Mills, P.C., and McMillan, W.D., 2004, Herbicides and their transformation products in source-

               water aquifers tapped by public-supply wells in Illinois, 2001-2002: U.S. Geological

               Survey Water-Resources Investigations Report 03-4226, 57 p.

       

Zimmerman, L.R., Hostetler, K.A., and Thurman, E.M., 2000, Method of analysis by the

               U.S. Geological Survey Organic Geochemistry Research Group - determination of

               chloroacetanilide herbicides in water using high-performance liquid chromatography-

               diode array detection and high-performance liquid chromatography/mass spectrometry:

               U.S. Geological Survey Open-File Report 00-182, 30 p.

 

 

 

 

               

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